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Yuan, Dafei; Awais, Mohammad A.; Sharapov, Valerii; Liu, Xunshan; Neshchadin, Andriy; Chen, Wei; Yu, Luping (, Journal of the American Chemical Society)null (Ed.)
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Yuan, Dafei; Awais, Mohammad A.; Sharapov, Valerii; Liu, Xunshan; Neshchadin, Andriy; Chen, Wei; Bera, Mrinal; Yu, Luping (, Chemical Science)null (Ed.)A critical issue in developing high-performance organic light-emitting transistors (OLETs) is to balance the trade-off between charge transport and light emission in a semiconducting material. Although traditional materials for organic light-emitting diodes (OLEDs) or organic field-effect transistors (OFETs) have shown modest performance in OLET devices, design strategies towards high-performance OLET materials and the crucial structure–performance relationship remain unclear. Our research effort in developing cross-conjugated weak acceptor-weak donor copolymers for luminescent properties lead us to an unintentional discovery that these copolymers form coiled foldamers with intramolecular H-aggregation, leading to their exceptional OLET properties. An impressive external quantum efficiency (EQE) of 6.9% in solution-processed multi-layer OLET devices was achieved.more » « less
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Yuan, Dafei; Awais, Mohammad A.; Sharapov, Valerii; Liu, Xunshan; Neshchadin, Andriy; Chen, Wei; Yu, Luping (, Chemistry of Materials)null (Ed.)
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Niklas, Jens; Zheng, Tianyue; Neshchadin, Andriy; Mardis, Kristy L.; Yu, Luping; Poluektov, Oleg G. (, Journal of the American Chemical Society)
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